Klein writes that sigla is probably related to the Aramaic segola סגולא, meaning cluster of grapes. He doesn't explain the connection - Jastrow suggests that sigla means "a bunch of violets". This term appears in Yerushalmi Peah 7, and Steinsaltz writes that it is an Aramaic variation of eshkol אשכול - also meaning a cluster of grapes. It appears in Targum Yonatan on Bamidbar 14:23 as a translation to eshkol. From segola we get the name of the vowel segol סגול - which also looks like a cluster of grapes.
What about the meaning of segula סגולה as treasure? Could the phrase am segula עם סגולה - mean "a purple nation"? While this site tries to establish a connection, I think it's not very likely. In fact, we have already seen that segula is related to the Akkadian sugullu - herd of cattle.
Rosenthal does not suggest any slang associations with the color sagol.
Update: I have since written a much more detailed post about segula. If you found this of interest, I suggest you continue and read that post as well.
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